Abstract
In the early days of quantum mechanics Kapitza and Dirac predicted that matter waves would scatter off the optical intensity grating formed by two counter-propagating light waves1. This interaction, driven by the ponderomotive potential of the optical standing wave, was both studied theoretically and demonstrated experimentally for atoms2 and electrons3,4,5. In the original version of the experiment1,5, only the transverse momentum of particles was varied, but their energy and longitudinal momentum remained unchanged after the interaction. Here, we report on the generalization of the Kapitza–Dirac effect. We demonstrate that the energy of sub-relativistic electrons is strongly modulated on the few-femtosecond timescale via the interaction with a travelling wave created in vacuum by two colliding laser pulses at different frequencies. This effect extends the possibilities of temporal control of freely propagating particles with coherent light and can serve the attosecond ballistic bunching of electrons6, or for the acceleration of neutral atoms or molecules by light.
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References
Kapitza, P. L. & Dirac, P. A. M. The reflection of electrons from standing light waves. Proc. Camb. Phil. Soc. 29, 297–300 (1933).
Gould, P. L., Ruff, G. A. & Pritchard, D. E. Diffraction of atoms by light: the near-resonant Kapitza–Dirac effect. Phys. Rev. Lett. 56, 827–830 (1986).
Bucksbaum, P. H., Bashkansky, M. & McIlrath, T. J. Scattering of electrons by intense coherent light. Phys. Rev. Lett. 58, 349–352 (1987).
Bucksbaum, P. H., Schumacher, D. W. & Bashkansky, M. High intensity Kapitza–Dirac effect. Phys. Rev. Lett. 61, 1182–1185 (1988).
Freimund, D. L., Aflatooni, K. & Batelaan, H. Observation of the Kapitza–Dirac effect. Nature 413, 142–143 (2001).
Baum, P. & Zewail, A. H. Attosecond electron pulses for 4D diffraction and microscopy. Proc. Natl Acad. Sci. USA 104, 18409–18414 (2007).
Batelaan, H. Colloquium: illuminating the Kapitza–Dirac effect with electron matter optics. Rev. Mod. Phys. 79, 929–941 (2007).
Efremov, M. A. & Fedorov, M. V. Classical and quantum versions of the Kapitza–Dirac effect. J. Exp. Theor. Phys. 89, 460–467 (1999).
Li, X. et al. Theory of the Kapitza–Dirac diffraction effect. Phys. Rev. Lett. 92, 233603 (2004).
Chan, Y. W. & Tsui, L. Classical theory of scattering of an electron beam by a laser standing wave. Phys. Rev. A 20, 294–303 (1979).
Freimund, D. L. & Batelaan, H. Bragg scattering of free electrons using the Kapitza–Dirac effect. Phys. Rev. Lett. 89, 283602 (2002).
Dellweg, M. M. & Müller, C. Kapitza–Dirac scattering of electrons from a bichromatic standing laser wave. Phys. Rev. A 91, 062102 (2015).
Smirnova, O., Freimund, D. L., Batelaan, H. & Ivanov, M. Kapitza–Dirac diffraction without standing waves: diffraction without a grating? Phys. Rev. Lett. 92, 223601 (2004).
Haroutunian, V. M. & Avetissian, H. K. An analogue of the Kapitza–Dirac effect. Phys. Lett. A 51, 320–322 (1975).
Varró, S. & Ehlotzky, F. Potential scattering of electrons in a bichromatic laser field of frequencies ω and 2ω or ω and 3ω. Opt. Commun. 99, 177–184 (1993).
Hilbert, S. A., Uiterwaal, C., Barwick, B., Batelaan, H. & Zewail, A. H. Temporal lenses for attosecond and femtosecond electron pulses. Proc. Natl Acad. Sci. USA 106, 10558–10563 (2009).
Baum, P. & Zewail, A. H. 4D attosecond imaging with free electrons: diffraction methods and potential applications. Chem. Phys. 366, 2–8 (2009).
Baum, P. On the physics of ultrashort single-electron pulses for time-resolved microscopy and diffraction. Chem. Phys. 423, 55–61 (2013).
Kozák, M. Electron acceleration in moving laser-induced gratings produced by chirped femtosecond pulses. J. Phys. B 48, 195601 (2015).
England, R. J. et al. Dielectric laser accelerators. Rev. Mod. Phys. 86, 1337–1389 (2014).
Carbajo, S. et al. Direct longitudinal laser acceleration of electrons in free space. Phys. Rev. Accel. Beams 19, 021303 (2016).
Peralta, E. A. et al. Demonstration of electron acceleration in a laser-driven dielectric microstructure. Nature 503, 91–94 (2013).
Breuer, J. & Hommelhoff, P. Laser-based acceleration of nonrelativistic electrons at a dielectric structure. Phys. Rev. Lett. 111, 134803 (2013).
Siwick, B. J., Dwyer, J. R., Jordan, R. E. & Miller, R. J. D. An atomic-level view of melting using femtosecond electron diffraction. Science 302, 1382–1385 (2003).
Baum, P. & Zewail, A. H. Breaking resolution limits in ultrafast electron diffraction and microscopy. Proc. Natl Acad. Sci. USA 103, 16105–16110 (2006).
Barwick, B., Flannigan, D. J. & Zewail, A. H. Photon-induced near-field electron microscopy. Nature 462, 902–906 (2009).
Piazza, L. et al. Simultaneous observation of the quantization and the interference pattern of a plasmonic near-field. Nat. Commun. 6, 6407 (2015).
Feist, A. et al. Quantum coherent optical phase modulation in an ultrafast transmission electron microscope. Nature 521, 200–203 (2015).
Echternkamp, K. E., Feist, A., Schäfer, S. & Ropers, C. Ramsey-type phase control of free-electron beams. Nat. Phys. 12, 1000–1004 (2016).
Kozák, M. et al. Optical gating and streaking of free-electrons with sub-optical-cycle precision. Nat. Commun. 8, 14342 (2017).
McGregor, S., Huang, W. C.-W., Shadwick, B. A. & Batelaan, H. Spin-dependent two-color Kapitza–Dirac effects. Phys. Rev. A 92, 023834 (2015).
Erhard, R. & Bauke, H. Spin effects in Kapitza–Dirac scattering at light with elliptical polarization. Phys. Rev. A 92, 042123 (2015).
Dellweg, M. M. & Müller, C. Spin-polarizing interferometric beam splitter for free electrons. Phys. Rev. Lett. 118, 070403 (2017).
Goodman, J. W. Introduction to Fourier Optics (McGraw-Hill, 1996).
Borggreen, J., Elbek, B. & Nielsen, L. P. A proposed spectrograph for heavy particles. Nucl. Instrum. Methods 24, 1–12 (1963).
Acknowledgements
We thank T. Higuchi and J. McNeur for proof-reading of the manuscript. The authors acknowledge funding from ERC grant ‘Near Field Atto’. This publication is funded in part by the Gordon and Betty Moore Foundation through Grant GBMF4744 ‘Accelerator on a Chip International Program – ACHIP’ and by BMBF via a project with contract number 05K16WEC.
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M.K. planned and carried out the experiments, processed the data and performed the simulations. T.E. designed and fabricated the electromagnetic spectrometer. N.S. developed the controlling software for data acquisition. M.K. and P.H. interpreted the results and wrote the manuscript with contributions of all authors.
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Kozák, M., Eckstein, T., Schönenberger, N. et al. Inelastic ponderomotive scattering of electrons at a high-intensity optical travelling wave in vacuum. Nat. Phys. 14, 121–125 (2018). https://doi.org/10.1038/nphys4282
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DOI: https://doi.org/10.1038/nphys4282


