Skip to main content

Thank you for visiting nature.com. You are using a browser version with limited support for CSS. To obtain the best experience, we recommend you use a more up to date browser (or turn off compatibility mode in Internet Explorer). In the meantime, to ensure continued support, we are displaying the site without styles and JavaScript.

  • Letter
  • Published:

Inelastic ponderomotive scattering of electrons at a high-intensity optical travelling wave in vacuum

Abstract

In the early days of quantum mechanics Kapitza and Dirac predicted that matter waves would scatter off the optical intensity grating formed by two counter-propagating light waves1. This interaction, driven by the ponderomotive potential of the optical standing wave, was both studied theoretically and demonstrated experimentally for atoms2 and electrons3,4,5. In the original version of the experiment1,5, only the transverse momentum of particles was varied, but their energy and longitudinal momentum remained unchanged after the interaction. Here, we report on the generalization of the Kapitza–Dirac effect. We demonstrate that the energy of sub-relativistic electrons is strongly modulated on the few-femtosecond timescale via the interaction with a travelling wave created in vacuum by two colliding laser pulses at different frequencies. This effect extends the possibilities of temporal control of freely propagating particles with coherent light and can serve the attosecond ballistic bunching of electrons6, or for the acceleration of neutral atoms or molecules by light.

This is a preview of subscription content, access via your institution

Access options

Access Nature and 54 other Nature Portfolio journals

Get Nature+, our best-value online-access subscription

$32.99 / 30 days cancel any time
Learn more

Buy this article

USD 39.95

Prices may be subject to local taxes which are calculated during checkout

Figure 1: Layout of the experiment demonstrating the inelastic ponderomotive scattering of electrons at a high-intensity optical travelling wave in vacuum.
Image
Figure 2: Measurements of electron spectra after the inelastic ponderomotive scattering at a high-intensity optical travelling wave in vacuum.
Image
Figure 3: Attosecond ballistic bunching of electrons after the interaction with the optical travelling wave.
Image

Similar content being viewed by others

References

  1. Kapitza, P. L. & Dirac, P. A. M. The reflection of electrons from standing light waves. Proc. Camb. Phil. Soc. 29, 297–300 (1933).

    Article  ADS  Google Scholar 

  2. Gould, P. L., Ruff, G. A. & Pritchard, D. E. Diffraction of atoms by light: the near-resonant Kapitza–Dirac effect. Phys. Rev. Lett. 56, 827–830 (1986).

    Article  ADS  Google Scholar 

  3. Bucksbaum, P. H., Bashkansky, M. & McIlrath, T. J. Scattering of electrons by intense coherent light. Phys. Rev. Lett. 58, 349–352 (1987).

    Article  ADS  Google Scholar 

  4. Bucksbaum, P. H., Schumacher, D. W. & Bashkansky, M. High intensity Kapitza–Dirac effect. Phys. Rev. Lett. 61, 1182–1185 (1988).

    Article  ADS  Google Scholar 

  5. Freimund, D. L., Aflatooni, K. & Batelaan, H. Observation of the Kapitza–Dirac effect. Nature 413, 142–143 (2001).

    Article  ADS  Google Scholar 

  6. Baum, P. & Zewail, A. H. Attosecond electron pulses for 4D diffraction and microscopy. Proc. Natl Acad. Sci. USA 104, 18409–18414 (2007).

    Article  ADS  Google Scholar 

  7. Batelaan, H. Colloquium: illuminating the Kapitza–Dirac effect with electron matter optics. Rev. Mod. Phys. 79, 929–941 (2007).

    Article  ADS  Google Scholar 

  8. Efremov, M. A. & Fedorov, M. V. Classical and quantum versions of the Kapitza–Dirac effect. J. Exp. Theor. Phys. 89, 460–467 (1999).

    Article  ADS  Google Scholar 

  9. Li, X. et al. Theory of the Kapitza–Dirac diffraction effect. Phys. Rev. Lett. 92, 233603 (2004).

    Article  ADS  Google Scholar 

  10. Chan, Y. W. & Tsui, L. Classical theory of scattering of an electron beam by a laser standing wave. Phys. Rev. A 20, 294–303 (1979).

    Article  ADS  Google Scholar 

  11. Freimund, D. L. & Batelaan, H. Bragg scattering of free electrons using the Kapitza–Dirac effect. Phys. Rev. Lett. 89, 283602 (2002).

    Article  ADS  Google Scholar 

  12. Dellweg, M. M. & Müller, C. Kapitza–Dirac scattering of electrons from a bichromatic standing laser wave. Phys. Rev. A 91, 062102 (2015).

    Article  ADS  Google Scholar 

  13. Smirnova, O., Freimund, D. L., Batelaan, H. & Ivanov, M. Kapitza–Dirac diffraction without standing waves: diffraction without a grating? Phys. Rev. Lett. 92, 223601 (2004).

    Article  ADS  Google Scholar 

  14. Haroutunian, V. M. & Avetissian, H. K. An analogue of the Kapitza–Dirac effect. Phys. Lett. A 51, 320–322 (1975).

    Article  ADS  Google Scholar 

  15. Varró, S. & Ehlotzky, F. Potential scattering of electrons in a bichromatic laser field of frequencies ω and 2ω or ω and 3ω. Opt. Commun. 99, 177–184 (1993).

    Article  ADS  Google Scholar 

  16. Hilbert, S. A., Uiterwaal, C., Barwick, B., Batelaan, H. & Zewail, A. H. Temporal lenses for attosecond and femtosecond electron pulses. Proc. Natl Acad. Sci. USA 106, 10558–10563 (2009).

    Article  ADS  Google Scholar 

  17. Baum, P. & Zewail, A. H. 4D attosecond imaging with free electrons: diffraction methods and potential applications. Chem. Phys. 366, 2–8 (2009).

    Article  Google Scholar 

  18. Baum, P. On the physics of ultrashort single-electron pulses for time-resolved microscopy and diffraction. Chem. Phys. 423, 55–61 (2013).

    Article  Google Scholar 

  19. Kozák, M. Electron acceleration in moving laser-induced gratings produced by chirped femtosecond pulses. J. Phys. B 48, 195601 (2015).

    Article  ADS  Google Scholar 

  20. England, R. J. et al. Dielectric laser accelerators. Rev. Mod. Phys. 86, 1337–1389 (2014).

    Article  ADS  Google Scholar 

  21. Carbajo, S. et al. Direct longitudinal laser acceleration of electrons in free space. Phys. Rev. Accel. Beams 19, 021303 (2016).

    Article  ADS  Google Scholar 

  22. Peralta, E. A. et al. Demonstration of electron acceleration in a laser-driven dielectric microstructure. Nature 503, 91–94 (2013).

    Article  ADS  Google Scholar 

  23. Breuer, J. & Hommelhoff, P. Laser-based acceleration of nonrelativistic electrons at a dielectric structure. Phys. Rev. Lett. 111, 134803 (2013).

    Article  ADS  Google Scholar 

  24. Siwick, B. J., Dwyer, J. R., Jordan, R. E. & Miller, R. J. D. An atomic-level view of melting using femtosecond electron diffraction. Science 302, 1382–1385 (2003).

    Article  ADS  Google Scholar 

  25. Baum, P. & Zewail, A. H. Breaking resolution limits in ultrafast electron diffraction and microscopy. Proc. Natl Acad. Sci. USA 103, 16105–16110 (2006).

    Article  ADS  Google Scholar 

  26. Barwick, B., Flannigan, D. J. & Zewail, A. H. Photon-induced near-field electron microscopy. Nature 462, 902–906 (2009).

    Article  ADS  Google Scholar 

  27. Piazza, L. et al. Simultaneous observation of the quantization and the interference pattern of a plasmonic near-field. Nat. Commun. 6, 6407 (2015).

    Article  ADS  Google Scholar 

  28. Feist, A. et al. Quantum coherent optical phase modulation in an ultrafast transmission electron microscope. Nature 521, 200–203 (2015).

    Article  ADS  Google Scholar 

  29. Echternkamp, K. E., Feist, A., Schäfer, S. & Ropers, C. Ramsey-type phase control of free-electron beams. Nat. Phys. 12, 1000–1004 (2016).

    Article  Google Scholar 

  30. Kozák, M. et al. Optical gating and streaking of free-electrons with sub-optical-cycle precision. Nat. Commun. 8, 14342 (2017).

    Article  ADS  Google Scholar 

  31. McGregor, S., Huang, W. C.-W., Shadwick, B. A. & Batelaan, H. Spin-dependent two-color Kapitza–Dirac effects. Phys. Rev. A 92, 023834 (2015).

    Article  ADS  Google Scholar 

  32. Erhard, R. & Bauke, H. Spin effects in Kapitza–Dirac scattering at light with elliptical polarization. Phys. Rev. A 92, 042123 (2015).

    Article  ADS  Google Scholar 

  33. Dellweg, M. M. & Müller, C. Spin-polarizing interferometric beam splitter for free electrons. Phys. Rev. Lett. 118, 070403 (2017).

    Article  ADS  Google Scholar 

  34. Goodman, J. W. Introduction to Fourier Optics (McGraw-Hill, 1996).

    Google Scholar 

  35. Borggreen, J., Elbek, B. & Nielsen, L. P. A proposed spectrograph for heavy particles. Nucl. Instrum. Methods 24, 1–12 (1963).

    Article  ADS  Google Scholar 

Download references

Acknowledgements

We thank T. Higuchi and J. McNeur for proof-reading of the manuscript. The authors acknowledge funding from ERC grant ‘Near Field Atto’. This publication is funded in part by the Gordon and Betty Moore Foundation through Grant GBMF4744 ‘Accelerator on a Chip International Program – ACHIP’ and by BMBF via a project with contract number 05K16WEC.

Author information

Authors and Affiliations

Authors

Contributions

M.K. planned and carried out the experiments, processed the data and performed the simulations. T.E. designed and fabricated the electromagnetic spectrometer. N.S. developed the controlling software for data acquisition. M.K. and P.H. interpreted the results and wrote the manuscript with contributions of all authors.

Corresponding author

Correspondence to M. Kozák.

Ethics declarations

Competing interests

The authors declare no competing financial interests.

Supplementary information

Supplementary information (download PDF )

Supplementary information (PDF 530 kb)

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Kozák, M., Eckstein, T., Schönenberger, N. et al. Inelastic ponderomotive scattering of electrons at a high-intensity optical travelling wave in vacuum. Nat. Phys. 14, 121–125 (2018). https://doi.org/10.1038/nphys4282

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue date:

  • DOI: https://doi.org/10.1038/nphys4282

Search

Quick links

Nature Briefing

Sign up for the Nature Briefing newsletter — what matters in science, free to your inbox daily.

Get the most important science stories of the day, free in your inbox. Sign up for Nature Briefing